Process the flour, cornmeal, sugar, and salt together in food processor until combined, about 5 seconds.
1 ⅓ cups all purpose flour, ⅓ cup yellow cornmeal, 2 tablespoons granulated sugar, ¼ teaspoon fine sea salt
Add the butter cubes to the flour mixture. Pulse until the mixture starts to clump together but is still sandy.
½ cup unsalted butter, cubed and cold
Stream in the buttermilk, pulsing in 4 second increments until the dough is moist and slightly sticky, but not wet, with no big pockets of dry flour remaining.
¼ cup buttermilk, cold
Turn the dough out onto a lightly floured or non-stick rolling mat. Form the dough into a disk shape, about 1 inch thick. Use a light hand to keep the butter from melting.
Wrap the dough tightly with plastic wrap and press down to flatten the disk. Refrigerate the dough for one hour or for up to three days.
Line a large cookie sheet with parchment paper. Preheat the oven to 400F.
Place the chilled dough on a lightly floured surface or a non-stick rolling mat. Roll from the center outward, rotating the dough 180 degrees, with your hands, every so often. This helps keep its round shape and prevents sticking. Add a little more flour if needed to prevent sticking.
Roll the dough to about ⅛" thick and about 12" round. Transfer the dough onto the parchment lined cookie sheet.
Chill for 20 minutes.